Tuesday, May 22, 2012

1205.4449 (Norio Takemoto et al.)

Phase Space Approach to Laser-driven Electronic Wavepacket Propagation    [PDF]

Norio Takemoto, Asaf Shimshovitz, David J. Tannor
We propose a phase space method to propagate a quantum wavepacket driven by a strong external field. The method employs the so-called biorthogonal von Neumann basis recently introduced for the calculation of the energy eigenstates of time-independent quantum systems [A. Shimshovitz and D.J. Tannor, arXiv:1201.2299v1]. While the individual elements in this basis set are time-independent, a small subset is chosen in a time-dependent manner to adapt to the evolution of the wavepacket in phase space. We demonstrate the accuracy and efficiency of the present propagation method by calculating the electronic wavepacket in a one-dimensional soft-core atom interacting with a superposition of an intense, few-cycle, near-infrared laser pulse and an attosecond extreme-ultraviolet laser pulse.
View original: http://arxiv.org/abs/1205.4449

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