J. M. Dahlström, D. Guénot, K. Klünder, M. Gisselbrecht, J. Mauritsson, A. L'Huillier, A. Maquet, R. Taïeb
We study the temporal aspects of laser-assisted extreme ultraviolet (XUV)
photoionization using attosecond pulses of harmonic radiation. The aim of this
paper is to establish the general form of the phase of the relevant transition
amplitudes and to make the connection with the time-delays that have been
recently measured in experiments. We find that the overall phase contains two
distinct types of contributions: one is expressed in terms of the phase-shifts
of the photoelectron continuum wavefunction while the other is linked to
continuum--continuum transitions induced by the infrared (IR) laser probe. Our
formalism applies to both kinds of measurements reported so far, namely the
ones using attosecond pulse trains of XUV harmonics and the others based on the
use of isolated attosecond pulses (streaking). The connection between the
phases and the time-delays is established with the help of finite difference
approximations to the energy derivatives of the phases. This makes clear that
the observed time-delays is a sum of two components: a one-photon Wigner-like
delay and an universal delay that originates from the probing process itself.
View original:
http://arxiv.org/abs/1112.4144
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