Li Zhang, Robert Hammond, Merav Dolev, Min Liu, Alexander Palevski, Aharon Kapitulnik
We report a novel method to fabricate high quality Bi2Se3 thin films using MBE with a radio frequency cracker cell as an atomic selenium source. With rates close to exact stoichiometry, optimal layer-by-layer growth of high quality Bi2Se3 thin films, with smooth surfaces, has been achieved on CaF2(111) substrates and Si(111) substrates with a thin CaF2 buffer layer(CaF2/Si). Transport measurements on these films show a characteristic weak antilocalization mangnetoresistance, with emergence of weak localization in the ultrathin film limit. Quantum Oscillations attributed to the topological surface states have been observed, including in films on CaF2/Si.
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http://arxiv.org/abs/1205.5832
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