1208.3997 (I. Siloi et al.)

Towards the chemical tuning of entanglement in molecular nanomagnets    [PDF]

I. Siloi, F. Troiani

Antiferromagnetic spin rings represent prototypical realizations of highly correlated, low-dimensional systems. Here we theoretically show how the introduction of magnetic defects by controlled chemical substitutions results in a strong spatial modulation of spin-pair entanglement within each ring. Entanglement between local degrees of freedom (individual spins) and collective ones (total ring spins) are shown to coexist in exchange-coupled ring dimers, as can be deduced from general symmetry arguments. We verify the persistence of these features at finite temperatures, and discuss them in terms of experimentally accessible observables.

View original: http://arxiv.org/abs/1208.3997